Vapor Transport Deposition of Metal-Halide Perovskites Solar Cells

Wan-Ju Hsu; Emma C. Pettit; Richard Swartwout; Tamar Kadosh; Shreyas Srinivasan; Ella L. Wassweiler; Vladimir Bulović; Russell J. Holmes

doi:10.1117/12.2677144

Vapor Transport Deposition of Metal-Halide Perovskites Solar Cells

Wan-Ju Hsu, Emma C. Pettit, Richard Swartwout, Tamar Kadosh, Shreyas Srinivasan, Ella L. Wassweiler, Vladimir Bulović, Russell J. Holmes

Chemical Engineering and Materials Science

Research output: Chapter in Book/Report/Conference proceeding › Conference contribution

Abstract

Photovoltaics based on metal-halide perovskites (MHPs) have exceeded the performance of other thin film technologies. However, there are challenges that frustrate the use of current MHP synthesis techniques for large-scale manufacturing. Here, efficient solar cells are demonstrated based on an active layer of methylammonium lead iodide (MAPbI₃) codeposited via vapor transport deposition (VTD). Our system design enables different source temperatures and carrier gas flow rates for the individual precursors, allowing precursor co-deposition and control over perovskite film composition. VTD-processed devices based on an active layer of MAPbI₃ realize power conversion efficiencies >10% under AM1.5G solar simulated illumination.

Original language	English (US)
Title of host publication	Organic, Hybrid, and Perovskite Photovoltaics XXIV
Editors	Gang Li, Natalie Stingelin, Ana Flavia Nogueira, Thuc-Quyen Nguyen, Ellen Moons, Barry P. Rand
Publisher	SPIE
ISBN (Electronic)	9781510665347
DOIs	https://doi.org/10.1117/12.2677144
State	Published - 2023
Event	Organic, Hybrid, and Perovskite Photovoltaics XXIV 2023 - San Diego, United States Duration: Aug 22 2023 → Aug 24 2023

Publication series

Name	Proceedings of SPIE - The International Society for Optical Engineering
Volume	12660
ISSN (Print)	0277-786X
ISSN (Electronic)	1996-756X

Conference

Conference	Organic, Hybrid, and Perovskite Photovoltaics XXIV 2023
Country/Territory	United States
City	San Diego
Period	8/22/23 → 8/24/23

Bibliographical note

Publisher Copyright:
© 2023 SPIE. All rights reserved.

Keywords

MAPbI
metal-halide perovskites
perovskite solar cells
vapor transport deposition

UN SDGs

This output contributes to the following UN Sustainable Development Goals (SDGs)

Publisher link

10.1117/12.2677144

Find It

Find It at U of M Libraries

Cite this

Hsu, W.-J., Pettit, E. C., Swartwout, R., Kadosh, T., Srinivasan, S., Wassweiler, E. L., Bulović, V., & Holmes, R. J. (2023). Vapor Transport Deposition of Metal-Halide Perovskites Solar Cells. In G. Li, N. Stingelin, A. F. Nogueira, T.-Q. Nguyen, E. Moons, & B. P. Rand (Eds.), Organic, Hybrid, and Perovskite Photovoltaics XXIV Article 1266007 (Proceedings of SPIE - The International Society for Optical Engineering; Vol. 12660). SPIE. https://doi.org/10.1117/12.2677144

Vapor Transport Deposition of Metal-Halide Perovskites Solar Cells. / Hsu, Wan-Ju; Pettit, Emma C.; Swartwout, Richard et al.
Organic, Hybrid, and Perovskite Photovoltaics XXIV. ed. / Gang Li; Natalie Stingelin; Ana Flavia Nogueira; Thuc-Quyen Nguyen; Ellen Moons; Barry P. Rand. SPIE, 2023. 1266007 (Proceedings of SPIE - The International Society for Optical Engineering; Vol. 12660).

Research output: Chapter in Book/Report/Conference proceeding › Conference contribution

Hsu, W-J, Pettit, EC, Swartwout, R, Kadosh, T, Srinivasan, S, Wassweiler, EL, Bulović, V & Holmes, RJ 2023, Vapor Transport Deposition of Metal-Halide Perovskites Solar Cells. in G Li, N Stingelin, AF Nogueira, T-Q Nguyen, E Moons & BP Rand (eds), Organic, Hybrid, and Perovskite Photovoltaics XXIV., 1266007, Proceedings of SPIE - The International Society for Optical Engineering, vol. 12660, SPIE, Organic, Hybrid, and Perovskite Photovoltaics XXIV 2023, San Diego, United States, 8/22/23. https://doi.org/10.1117/12.2677144

Hsu WJ, Pettit EC, Swartwout R, Kadosh T, Srinivasan S, Wassweiler EL et al. Vapor Transport Deposition of Metal-Halide Perovskites Solar Cells. In Li G, Stingelin N, Nogueira AF, Nguyen TQ, Moons E, Rand BP, editors, Organic, Hybrid, and Perovskite Photovoltaics XXIV. SPIE. 2023. 1266007. (Proceedings of SPIE - The International Society for Optical Engineering). doi: 10.1117/12.2677144

Hsu, Wan-Ju ; Pettit, Emma C. ; Swartwout, Richard et al. / Vapor Transport Deposition of Metal-Halide Perovskites Solar Cells. Organic, Hybrid, and Perovskite Photovoltaics XXIV. editor / Gang Li ; Natalie Stingelin ; Ana Flavia Nogueira ; Thuc-Quyen Nguyen ; Ellen Moons ; Barry P. Rand. SPIE, 2023. (Proceedings of SPIE - The International Society for Optical Engineering).

@inproceedings{1c705e62082949c681578188e9659463,

title = "Vapor Transport Deposition of Metal-Halide Perovskites Solar Cells",

abstract = "Photovoltaics based on metal-halide perovskites (MHPs) have exceeded the performance of other thin film technologies. However, there are challenges that frustrate the use of current MHP synthesis techniques for large-scale manufacturing. Here, efficient solar cells are demonstrated based on an active layer of methylammonium lead iodide (MAPbI3) codeposited via vapor transport deposition (VTD). Our system design enables different source temperatures and carrier gas flow rates for the individual precursors, allowing precursor co-deposition and control over perovskite film composition. VTD-processed devices based on an active layer of MAPbI3 realize power conversion efficiencies >10% under AM1.5G solar simulated illumination.",

keywords = "MAPbI, metal-halide perovskites, perovskite solar cells, vapor transport deposition",

author = "Wan-Ju Hsu and Pettit, {Emma C.} and Richard Swartwout and Tamar Kadosh and Shreyas Srinivasan and Wassweiler, {Ella L.} and Vladimir Bulovi{\'c} and Holmes, {Russell J.}",

year = "2023",

doi = "10.1117/12.2677144",

language = "English (US)",

series = "Proceedings of SPIE - The International Society for Optical Engineering",

publisher = "SPIE",

editor = "Gang Li and Natalie Stingelin and Nogueira, {Ana Flavia} and Thuc-Quyen Nguyen and Ellen Moons and Rand, {Barry P.}",

booktitle = "Organic, Hybrid, and Perovskite Photovoltaics XXIV",

address = "United States",

}

TY - GEN

T1 - Vapor Transport Deposition of Metal-Halide Perovskites Solar Cells

AU - Hsu, Wan-Ju

AU - Pettit, Emma C.

AU - Swartwout, Richard

AU - Kadosh, Tamar

AU - Srinivasan, Shreyas

AU - Wassweiler, Ella L.

AU - Bulović, Vladimir

AU - Holmes, Russell J.

PY - 2023

Y1 - 2023

N2 - Photovoltaics based on metal-halide perovskites (MHPs) have exceeded the performance of other thin film technologies. However, there are challenges that frustrate the use of current MHP synthesis techniques for large-scale manufacturing. Here, efficient solar cells are demonstrated based on an active layer of methylammonium lead iodide (MAPbI3) codeposited via vapor transport deposition (VTD). Our system design enables different source temperatures and carrier gas flow rates for the individual precursors, allowing precursor co-deposition and control over perovskite film composition. VTD-processed devices based on an active layer of MAPbI3 realize power conversion efficiencies >10% under AM1.5G solar simulated illumination.

AB - Photovoltaics based on metal-halide perovskites (MHPs) have exceeded the performance of other thin film technologies. However, there are challenges that frustrate the use of current MHP synthesis techniques for large-scale manufacturing. Here, efficient solar cells are demonstrated based on an active layer of methylammonium lead iodide (MAPbI3) codeposited via vapor transport deposition (VTD). Our system design enables different source temperatures and carrier gas flow rates for the individual precursors, allowing precursor co-deposition and control over perovskite film composition. VTD-processed devices based on an active layer of MAPbI3 realize power conversion efficiencies >10% under AM1.5G solar simulated illumination.

KW - MAPbI

KW - metal-halide perovskites

KW - perovskite solar cells

KW - vapor transport deposition

UR - http://www.scopus.com/inward/record.url?scp=85176499987&partnerID=8YFLogxK

UR - http://www.scopus.com/inward/citedby.url?scp=85176499987&partnerID=8YFLogxK

U2 - 10.1117/12.2677144

DO - 10.1117/12.2677144

M3 - Conference contribution

AN - SCOPUS:85176499987

T3 - Proceedings of SPIE - The International Society for Optical Engineering

BT - Organic, Hybrid, and Perovskite Photovoltaics XXIV

A2 - Li, Gang

A2 - Stingelin, Natalie

A2 - Nogueira, Ana Flavia

A2 - Nguyen, Thuc-Quyen

A2 - Moons, Ellen

A2 - Rand, Barry P.

PB - SPIE

T2 - Organic, Hybrid, and Perovskite Photovoltaics XXIV 2023

Y2 - 22 August 2023 through 24 August 2023

ER -

Vapor Transport Deposition of Metal-Halide Perovskites Solar Cells

Abstract

Publication series

Conference

Bibliographical note

Keywords

UN SDGs

Publisher link

Find It

Other files and links

Fingerprint

Cite this