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Abstract
Low-dimensional materials hold great promises for exploring emergent physical phenomena, nanoelectronics, and quantum technologies. Their synthesis often depends on catalytic metal films, from which the synthesized materials must be transferred to insulating substrates to enable device functionality and minimize interfacial interactions during quantum investigations. Conventional transfer methods, such as chemical etching or electrochemical delamination, degrade material quality, limit scalability, or prove incompatible with complex device architectures. Here, a scalable, etch-free transfer technique is presented, employing Field's metal (51% In, 32.5% Bi, and 16.5% Sn by weight) as a low-melting-point mechanical support to gently delaminate low-dimensional materials from metal films without causing damage. Anchoring the metal film during separation prevents tearing and preserves material integrity. As a proof of concept, atomically precise graphene nanoribbons (GNRs) are transferred from Au(111)/mica to dielectric substrates, including silicon dioxide (SiO2) and single-crystalline lanthanum oxychloride (LaOCl). Comprehensive characterization confirms the preservation of structural and chemical integrity throughout the transfer process. Wafer-scale compatibility and device integration are demonstrated by fabricating GNR-based field-effect transistors (GNRFETs) that exhibit room-temperature switching with on/off current ratios exceeding 103. This method provides a scalable and versatile platform for integrating low-dimensional materials into advanced low-dimensional materials-based technologies.
| Original language | English (US) |
|---|---|
| Article number | e00630 |
| Journal | Advanced Materials Interfaces |
| Volume | 13 |
| Issue number | 1 |
| DOIs | |
| State | Published - Jan 7 2026 |
Bibliographical note
Publisher Copyright:© 2025 The Author(s). Advanced Materials Interfaces published by Wiley-VCH GmbH.
Keywords
- 2D dielectrics
- etch-free transfer
- graphene nanoribbons
- low-dimensional materials
- Van der Waals heterostructures
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University of Minnesota Materials Research Science and Engineering Center (DMR-2011401)
Bates, F. S. (PI), Calabrese, M. A. (PI), Ellison, C. J. (PI), Ferry, V. E. (PI), Flannigan, D. J. (PI), Frisbie, D. (PI), Frontiera, R. R. (PI), Greven, M. (PI), Haynes, C. L. (PI), Head-Marsden, K. M. (PI), Ilic, O. (PI), Jalan, B. (PI), Lamb, J. R. (PI), Leighton, C. (PI), Lodge, T. (PI), Low, T. (PI), Mahanthappa, M. (PI), Mkhoyan, A. (PI), Reineke, T. M. (PI), Roman, A. J. (PI), Sarupria, S. (PI), Stoerzinger, K. A. (PI), Walker, L. M. (PI), Wang, X. (PI), Xiong, B. (PI), Holmes, R. J. (Key Personnel), Oh, S.-H. (Key Personnel), Martiniani, S. (Prior Principal Investigator) & Wang, K. (Prior Principal Investigator)
THE NATIONAL SCIENCE FOUNDATION
9/1/20 → 8/31/26
Project: Research project
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