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Scalable Etch-Free Transfer of Low-Dimensional Materials From Metal Films to Diverse Substrates

  • Kentaro Yumigeta
  • , Muhammed Yusufoglu
  • , Mamun Sarker
  • , Rishi Raj
  • , Franco Daluisio
  • , Richard Holloway
  • , Howard Yawit
  • , Thomas Sweepe
  • , Julian Battaglia
  • , Shelby Janssen
  • , Alex C. Welch
  • , Paul DiPasquale
  • , K. Andre Mkhoyan
  • , Alexander Sinitskii
  • , Zafer Mutlu

Research output: Contribution to journalArticlepeer-review

Abstract

Low-dimensional materials hold great promises for exploring emergent physical phenomena, nanoelectronics, and quantum technologies. Their synthesis often depends on catalytic metal films, from which the synthesized materials must be transferred to insulating substrates to enable device functionality and minimize interfacial interactions during quantum investigations. Conventional transfer methods, such as chemical etching or electrochemical delamination, degrade material quality, limit scalability, or prove incompatible with complex device architectures. Here, a scalable, etch-free transfer technique is presented, employing Field's metal (51% In, 32.5% Bi, and 16.5% Sn by weight) as a low-melting-point mechanical support to gently delaminate low-dimensional materials from metal films without causing damage. Anchoring the metal film during separation prevents tearing and preserves material integrity. As a proof of concept, atomically precise graphene nanoribbons (GNRs) are transferred from Au(111)/mica to dielectric substrates, including silicon dioxide (SiO2) and single-crystalline lanthanum oxychloride (LaOCl). Comprehensive characterization confirms the preservation of structural and chemical integrity throughout the transfer process. Wafer-scale compatibility and device integration are demonstrated by fabricating GNR-based field-effect transistors (GNRFETs) that exhibit room-temperature switching with on/off current ratios exceeding 103. This method provides a scalable and versatile platform for integrating low-dimensional materials into advanced low-dimensional materials-based technologies.

Original languageEnglish (US)
Article numbere00630
JournalAdvanced Materials Interfaces
Volume13
Issue number1
DOIs
StatePublished - Jan 7 2026

Bibliographical note

Publisher Copyright:
© 2025 The Author(s). Advanced Materials Interfaces published by Wiley-VCH GmbH.

Keywords

  • 2D dielectrics
  • etch-free transfer
  • graphene nanoribbons
  • low-dimensional materials
  • Van der Waals heterostructures

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