Abstract
The tensor elements of the direct fifth-order Raman signal from CS2 were collected and analyzed. The collection of results reduce contamination from third-order cascade signals that are of varying importance in different tensor elements. As predicted, the different tensor elements weight particular Liouville pathways of the direct fifth-order signal undergoing molecular dynamics.
Original language | English (US) |
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Pages (from-to) | 2312-2331 |
Number of pages | 20 |
Journal | Journal of Chemical Physics |
Volume | 114 |
Issue number | 5 |
DOIs | |
State | Published - 2001 |