Magnon-spinon dichotomy in the Kitaev hyperhoneycomb β-Li2IrO3

Alejandro Ruiz, Nicholas P. Breznay, Mengqun Li, Ioannis Rousochatzakis, Anthony Allen, Isaac Zinda, Vikram Nagarajan, Gilbert Lopez, Zahirul Islam, Mary H. Upton, Jungho Kim, Ayman H. Said, Xian Rong Huang, Thomas Gog, Diego Casa, Robert J. Birgeneau, Jake D. Koralek, James G. Analytis, Natalia B. Perkins, Alex Frano

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The family of edge-sharing tricoordinated iridates and ruthenates has emerged in recent years as a major platform for Kitaev spin-liquid physics, where spins fractionalize into emergent magnetic fluxes and Majorana fermions with Dirac-like dispersions. While such exotic states are usually preempted by long-range magnetic order at low temperatures, signatures of Majorana fermions with long coherent times have been predicted to manifest at intermediate and higher energy scales, similar to the observation of spinons in quasi-one-dimensional spin chains. Here we present a resonant inelastic X-ray scattering study of the magnetic excitations of the hyperhoneycomb iridate β-Li2IrO3 under a magnetic field with a record-high-resolution spectrometer. At low temperatures, dispersing spin waves can be resolved around the predicted intertwined incommensurate spiral and field-induced zigzag orders, whose excitation energy reaches a maximum of 16 meV. A 2 T magnetic field softens the dispersion around Q=0. The behavior of the spin waves under magnetic field is consistent with our semiclassical calculations for the ground state and the dynamical spin structure factor, which further predicts that the ensued intertwined uniform states remain robust up to very high fields (100 T). Most saliently, the low-energy magnonlike mode is superimposed by a broad continuum of excitations, centered around 35 meV and extending up to 100 meV. This high-energy continuum survives up to at least 300 K-well above the ordering temperature of 38 K- A nd gives evidence for pairs of long-lived Majorana fermions of the proximate Kitaev spin liquid.

Original languageEnglish (US)
Article number184404
JournalPhysical Review B
Issue number18
StatePublished - May 4 2021

Bibliographical note

Funding Information:
We thank Yi-Zhuang You, Tarun Grover, John McGreevy, Dan Arovas, Ken Burch, Yiping Wang, and Gabor Halasz for fruitful discussions. Use of the Advanced Photon Source was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. Synthesis was supported by the Department of Energy Early Career program, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, under Contract No. DE-AC02-05CH11231. The work at LBNL is funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division under Contract No. DE-AC02-05-CH11231 within the Quantum Materials Program (KC2202). Jake Koralek is supported by the U.S. Department of Energy, Office of Sciences, Office of Basic Energy Sciences under Contract No. DE-AC02-76SF00515. Alejandro Ruiz acknowledges support from the University of California President's Postdoctoral Fellowship Program. Natalia B. Perkins and Mengqun Li were supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences under Award No. DE-SC0018056. N.P.B. and I.Z. acknowledge the support of Harvey Mudd College. A.F. acknowledges support from the Alfred P. Sloan Fellowship in Physics.

Publisher Copyright:
© 2021 American Physical Society.


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