Abstract
We present an approach to study the ground-state and elementary excitations in compounds where spins and orbitals are entangled by on-site relativistic spin-orbit interaction. The appropriate degrees of freedom are localized states with an effective angular momentum J. We generalize J to arbitrary large values while maintaining the delicate spin-orbital entanglement. After projecting the intersite exchange interaction to the manifold of effective spins, a systematic 1/J expansion of the effective Hamiltonian is realized using the Holstein-Primakoff transformation. Applications to representative compounds Sr2 IrO4 and particularly vanadium spinels A V2 O4 are discussed.
| Original language | English (US) |
|---|---|
| Article number | 180409 |
| Journal | Physical Review B - Condensed Matter and Materials Physics |
| Volume | 80 |
| Issue number | 18 |
| DOIs | |
| State | Published - Nov 11 2009 |
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