High performance high-power textured Mn/Cu-doped PIN-PMN-PT ceramics

Haoyang Leng; Yongke Yan; Bo Wang; Tiannan Yang; Hairui Liu; Xiaotian Li; Rammohan Sriramdas; Ke Wang; Mark Fanton; Richard J. Meyer; Long Qing Chen; Shashank Priya

doi:10.1016/j.actamat.2022.118015

High performance high-power textured Mn/Cu-doped PIN-PMN-PT ceramics

Haoyang Leng, Yongke Yan, Bo Wang, Tiannan Yang, Hairui Liu, Xiaotian Li, Rammohan Sriramdas, Ke Wang, Mark Fanton, Richard J. Meyer, Long Qing Chen, Shashank Priya

Administration (RIO)

Research output: Contribution to journal › Article › peer-review

38 Scopus citations

Abstract

Piezoelectric ceramics with combinatory soft and hard characteristics are highly desired for high-power applications. However, it remains grand challenge to achieve simultaneous presence of hard (e.g. high coercive field, E_c; high mechanical quality factor, Q_m) and soft (e.g. high piezoelectric constant, d; high electromechanical coupling factor, k) piezoelectric properties in piezoelectric ceramics since the mechanism controlling the hard behavior (pinned domain walls) will significantly reduce the soft behavior. Here, we address this grand challenge and demonstrate <001> textured MnO₂ and CuO co-doped Pb(In_1/2Nb_1/2)O₃- Pb(Mg_1/3Nb_2/3)O₃-PbTiO₃ (PIN-PMN-PT) ceramics exhibiting ultrahigh combined soft and hard piezoelectric properties (d₃₃ = 713 pC N⁻¹, k₃₁ = 0.52, Q_m≈950, E_c = 9.6 kV cm⁻¹, tan δ = 0.45%). The outstanding electromechanical properties are explained by considering composition/phase selection, crystallographic anisotropy and defect engineering. Phase-field model in conjunction with high resolution electron microscopy and diffraction techniques is utilized to delineate the contributions arising from intrinsic piezoelectric response, domain dynamics, and local structural heterogeneity. These results will have significant impact in the development of high-power transducers and actuators.

Original language	English (US)
Article number	118015
Journal	Acta Materialia
Volume	234
DOIs	https://doi.org/10.1016/j.actamat.2022.118015
State	Published - Aug 1 2022

Bibliographical note

Funding Information:
H.L. and Y.Y. acknowledge the financial support from DARPA through award number HR00111920001 . H. Liu acknowledges the financial support from National Science Foundation through CREST CREAM program at Norfolk State University. T.Y. and L.-Q.C. are supported as part of the Computational Materials Sciences Program funded by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, under Award No. DE-SC0020145. B.W. acknowledges support by the National Science Foundation (NSF) through Grant No. DMR-1744213. X.L. acknowledges the financial support from Army Research Office through TE3 program ( W911NF1620010 ). S.P. acknowledges the financial support from National Science Foundation through the award number 1936432 . The computer simulations were performed using the commercial software package μ-PRO (http://mupro.co/contact/) on the ICS-ACI Computing Systems at Pennsylvania State University and at the Extreme Science and Engineering Discovery Environment cluster, which used the Comet system at the UC San Diego. We thank Haiying Wang for TEM sample preparation by using FIB. All microscopy work was performed at Penn State Materials Characterization Laboratory. The authors thank Dr. Harold Robinson, ONR Transduction Materials Project Manager, for constructive discussions of the results that has helped us in improving the quality of presentation.

Funding Information:
H.L. and Y.Y. acknowledge the financial support from DARPA through award number HR00111920001. H. Liu acknowledges the financial support from National Science Foundation through CREST CREAM program at Norfolk State University. T.Y. and L.-Q.C. are supported as part of the Computational Materials Sciences Program funded by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, under Award No. DE-SC0020145. B.W. acknowledges support by the National Science Foundation (NSF) through Grant No. DMR-1744213. X.L. acknowledges the financial support from Army Research Office through TE3 program (W911NF1620010). S.P. acknowledges the financial support from National Science Foundation through the award number 1936432. The computer simulations were performed using the commercial software package μ-PRO (http://mupro.co/contact/) on the ICS-ACI Computing Systems at Pennsylvania State University and at the Extreme Science and Engineering Discovery Environment cluster, which used the Comet system at the UC San Diego. We thank Haiying Wang for TEM sample preparation by using FIB. All microscopy work was performed at Penn State Materials Characterization Laboratory. The authors thank Dr. Harold Robinson, ONR Transduction Materials Project Manager, for constructive discussions of the results that has helped us in improving the quality of presentation.

Publisher Copyright:
© 2022 Acta Materialia Inc.

Keywords

Acceptor
Crystallography
High power
Piezoelectric
Texturing

Publisher link

10.1016/j.actamat.2022.118015

Find It

Find It at U of M Libraries

Cite this

@article{a30c55d698c6464da221313f0f218961,

title = "High performance high-power textured Mn/Cu-doped PIN-PMN-PT ceramics",

abstract = "Piezoelectric ceramics with combinatory soft and hard characteristics are highly desired for high-power applications. However, it remains grand challenge to achieve simultaneous presence of hard (e.g. high coercive field, Ec; high mechanical quality factor, Qm) and soft (e.g. high piezoelectric constant, d; high electromechanical coupling factor, k) piezoelectric properties in piezoelectric ceramics since the mechanism controlling the hard behavior (pinned domain walls) will significantly reduce the soft behavior. Here, we address this grand challenge and demonstrate <001> textured MnO2 and CuO co-doped Pb(In1/2Nb1/2)O3- Pb(Mg1/3Nb2/3)O3-PbTiO3 (PIN-PMN-PT) ceramics exhibiting ultrahigh combined soft and hard piezoelectric properties (d33 = 713 pC N−1, k31 = 0.52, Qm≈950, Ec = 9.6 kV cm−1, tan δ = 0.45%). The outstanding electromechanical properties are explained by considering composition/phase selection, crystallographic anisotropy and defect engineering. Phase-field model in conjunction with high resolution electron microscopy and diffraction techniques is utilized to delineate the contributions arising from intrinsic piezoelectric response, domain dynamics, and local structural heterogeneity. These results will have significant impact in the development of high-power transducers and actuators.",

keywords = "Acceptor, Crystallography, High power, Piezoelectric, Texturing",

author = "Haoyang Leng and Yongke Yan and Bo Wang and Tiannan Yang and Hairui Liu and Xiaotian Li and Rammohan Sriramdas and Ke Wang and Mark Fanton and Meyer, {Richard J.} and Chen, {Long Qing} and Shashank Priya",

note = "Funding Information: H.L. and Y.Y. acknowledge the financial support from DARPA through award number HR00111920001 . H. Liu acknowledges the financial support from National Science Foundation through CREST CREAM program at Norfolk State University. T.Y. and L.-Q.C. are supported as part of the Computational Materials Sciences Program funded by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, under Award No. DE-SC0020145. B.W. acknowledges support by the National Science Foundation (NSF) through Grant No. DMR-1744213. X.L. acknowledges the financial support from Army Research Office through TE3 program ( W911NF1620010 ). S.P. acknowledges the financial support from National Science Foundation through the award number 1936432 . The computer simulations were performed using the commercial software package μ-PRO (http://mupro.co/contact/) on the ICS-ACI Computing Systems at Pennsylvania State University and at the Extreme Science and Engineering Discovery Environment cluster, which used the Comet system at the UC San Diego. We thank Haiying Wang for TEM sample preparation by using FIB. All microscopy work was performed at Penn State Materials Characterization Laboratory. The authors thank Dr. Harold Robinson, ONR Transduction Materials Project Manager, for constructive discussions of the results that has helped us in improving the quality of presentation. Funding Information: H.L. and Y.Y. acknowledge the financial support from DARPA through award number HR00111920001. H. Liu acknowledges the financial support from National Science Foundation through CREST CREAM program at Norfolk State University. T.Y. and L.-Q.C. are supported as part of the Computational Materials Sciences Program funded by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, under Award No. DE-SC0020145. B.W. acknowledges support by the National Science Foundation (NSF) through Grant No. DMR-1744213. X.L. acknowledges the financial support from Army Research Office through TE3 program (W911NF1620010). S.P. acknowledges the financial support from National Science Foundation through the award number 1936432. The computer simulations were performed using the commercial software package μ-PRO (http://mupro.co/contact/) on the ICS-ACI Computing Systems at Pennsylvania State University and at the Extreme Science and Engineering Discovery Environment cluster, which used the Comet system at the UC San Diego. We thank Haiying Wang for TEM sample preparation by using FIB. All microscopy work was performed at Penn State Materials Characterization Laboratory. The authors thank Dr. Harold Robinson, ONR Transduction Materials Project Manager, for constructive discussions of the results that has helped us in improving the quality of presentation. Publisher Copyright: {\textcopyright} 2022 Acta Materialia Inc.",

year = "2022",

month = aug,

day = "1",

doi = "10.1016/j.actamat.2022.118015",

language = "English (US)",

volume = "234",

journal = "Acta Materialia",

issn = "1359-6454",

publisher = "Acta Materialia Inc",

}

TY - JOUR

T1 - High performance high-power textured Mn/Cu-doped PIN-PMN-PT ceramics

AU - Leng, Haoyang

AU - Yan, Yongke

AU - Wang, Bo

AU - Yang, Tiannan

AU - Liu, Hairui

AU - Li, Xiaotian

AU - Sriramdas, Rammohan

AU - Wang, Ke

AU - Fanton, Mark

AU - Meyer, Richard J.

AU - Chen, Long Qing

AU - Priya, Shashank

N1 - Funding Information: H.L. and Y.Y. acknowledge the financial support from DARPA through award number HR00111920001 . H. Liu acknowledges the financial support from National Science Foundation through CREST CREAM program at Norfolk State University. T.Y. and L.-Q.C. are supported as part of the Computational Materials Sciences Program funded by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, under Award No. DE-SC0020145. B.W. acknowledges support by the National Science Foundation (NSF) through Grant No. DMR-1744213. X.L. acknowledges the financial support from Army Research Office through TE3 program ( W911NF1620010 ). S.P. acknowledges the financial support from National Science Foundation through the award number 1936432 . The computer simulations were performed using the commercial software package μ-PRO (http://mupro.co/contact/) on the ICS-ACI Computing Systems at Pennsylvania State University and at the Extreme Science and Engineering Discovery Environment cluster, which used the Comet system at the UC San Diego. We thank Haiying Wang for TEM sample preparation by using FIB. All microscopy work was performed at Penn State Materials Characterization Laboratory. The authors thank Dr. Harold Robinson, ONR Transduction Materials Project Manager, for constructive discussions of the results that has helped us in improving the quality of presentation. Funding Information: H.L. and Y.Y. acknowledge the financial support from DARPA through award number HR00111920001. H. Liu acknowledges the financial support from National Science Foundation through CREST CREAM program at Norfolk State University. T.Y. and L.-Q.C. are supported as part of the Computational Materials Sciences Program funded by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, under Award No. DE-SC0020145. B.W. acknowledges support by the National Science Foundation (NSF) through Grant No. DMR-1744213. X.L. acknowledges the financial support from Army Research Office through TE3 program (W911NF1620010). S.P. acknowledges the financial support from National Science Foundation through the award number 1936432. The computer simulations were performed using the commercial software package μ-PRO (http://mupro.co/contact/) on the ICS-ACI Computing Systems at Pennsylvania State University and at the Extreme Science and Engineering Discovery Environment cluster, which used the Comet system at the UC San Diego. We thank Haiying Wang for TEM sample preparation by using FIB. All microscopy work was performed at Penn State Materials Characterization Laboratory. The authors thank Dr. Harold Robinson, ONR Transduction Materials Project Manager, for constructive discussions of the results that has helped us in improving the quality of presentation. Publisher Copyright: © 2022 Acta Materialia Inc.

PY - 2022/8/1

Y1 - 2022/8/1

N2 - Piezoelectric ceramics with combinatory soft and hard characteristics are highly desired for high-power applications. However, it remains grand challenge to achieve simultaneous presence of hard (e.g. high coercive field, Ec; high mechanical quality factor, Qm) and soft (e.g. high piezoelectric constant, d; high electromechanical coupling factor, k) piezoelectric properties in piezoelectric ceramics since the mechanism controlling the hard behavior (pinned domain walls) will significantly reduce the soft behavior. Here, we address this grand challenge and demonstrate <001> textured MnO2 and CuO co-doped Pb(In1/2Nb1/2)O3- Pb(Mg1/3Nb2/3)O3-PbTiO3 (PIN-PMN-PT) ceramics exhibiting ultrahigh combined soft and hard piezoelectric properties (d33 = 713 pC N−1, k31 = 0.52, Qm≈950, Ec = 9.6 kV cm−1, tan δ = 0.45%). The outstanding electromechanical properties are explained by considering composition/phase selection, crystallographic anisotropy and defect engineering. Phase-field model in conjunction with high resolution electron microscopy and diffraction techniques is utilized to delineate the contributions arising from intrinsic piezoelectric response, domain dynamics, and local structural heterogeneity. These results will have significant impact in the development of high-power transducers and actuators.

AB - Piezoelectric ceramics with combinatory soft and hard characteristics are highly desired for high-power applications. However, it remains grand challenge to achieve simultaneous presence of hard (e.g. high coercive field, Ec; high mechanical quality factor, Qm) and soft (e.g. high piezoelectric constant, d; high electromechanical coupling factor, k) piezoelectric properties in piezoelectric ceramics since the mechanism controlling the hard behavior (pinned domain walls) will significantly reduce the soft behavior. Here, we address this grand challenge and demonstrate <001> textured MnO2 and CuO co-doped Pb(In1/2Nb1/2)O3- Pb(Mg1/3Nb2/3)O3-PbTiO3 (PIN-PMN-PT) ceramics exhibiting ultrahigh combined soft and hard piezoelectric properties (d33 = 713 pC N−1, k31 = 0.52, Qm≈950, Ec = 9.6 kV cm−1, tan δ = 0.45%). The outstanding electromechanical properties are explained by considering composition/phase selection, crystallographic anisotropy and defect engineering. Phase-field model in conjunction with high resolution electron microscopy and diffraction techniques is utilized to delineate the contributions arising from intrinsic piezoelectric response, domain dynamics, and local structural heterogeneity. These results will have significant impact in the development of high-power transducers and actuators.

KW - Acceptor

KW - Crystallography

KW - High power

KW - Piezoelectric

KW - Texturing

UR - http://www.scopus.com/inward/record.url?scp=85130339443&partnerID=8YFLogxK

UR - http://www.scopus.com/inward/citedby.url?scp=85130339443&partnerID=8YFLogxK

U2 - 10.1016/j.actamat.2022.118015

DO - 10.1016/j.actamat.2022.118015

M3 - Article

AN - SCOPUS:85130339443

SN - 1359-6454

VL - 234

JO - Acta Materialia

JF - Acta Materialia

M1 - 118015

ER -

High performance high-power textured Mn/Cu-doped PIN-PMN-PT ceramics

Abstract

Bibliographical note

Keywords

Publisher link

Find It

Other files and links

Fingerprint

Cite this