Giant strain with ultra-low hysteresis and high temperature stability in grain oriented lead-free K 0.5 Bi 0.5 TiO3-BaTiO3-Na0.5 Bi0.5 TiO3 piezoelectric materials

Deepam Maurya; Yuan Zhou; Yaojin Wang; Yongke Yan; Jiefang Li; Dwight Viehland; Shashank Priya

doi:10.1038/srep08595

Giant strain with ultra-low hysteresis and high temperature stability in grain oriented lead-free K _0.5 Bi _0.5 TiO₃-BaTiO₃-Na_0.5 Bi_0.5 TiO₃ piezoelectric materials

Deepam Maurya, Yuan Zhou, Yaojin Wang, Yongke Yan, Jiefang Li, Dwight Viehland, Shashank Priya

Research output: Contribution to journal › Article › peer-review

106 Scopus citations

Abstract

We synthesized grain-oriented lead-free piezoelectric materials in (K _0.5 Bi _0.5 TiO₃-BaTiO₃-Na_0.5 Bi_0.5 TiO₃ (KBT-BT-NBT) system with high degree of texturing along the [001]c (c-cubic) crystallographic orientation. We demonstrate giant field induced strain (∼0.48%) with an ultra-low hysteresis along with enhanced piezoelectric response (d 33 ∼ 190pC/N) and high temperature stability (∼160°C). Transmission electron microscopy (TEM) and piezoresponse force microscopy (PFM) results demonstrate smaller size highly ordered domain structure in grain-oriented specimen relative to the conventional polycrystalline ceramics. The grain oriented specimens exhibited a high degree of non-180° domain switching, in comparison to the randomly axed ones. These results indicate the effective solution to the lead-free piezoelectric materials.

Original language	English (US)
Article number	8595
Journal	Scientific reports
Volume	5
DOIs	https://doi.org/10.1038/srep08595
State	Published - 2015
Externally published	Yes

Bibliographical note

Funding Information:
The authors gratefully acknowledge financial support from the Office of Basic Energy Science, Department of Energy through grant number DE-FG02-07ER46480. Thanks to Keyur B. Joshi for his help in calculating dissipated energy from the P-E hysteresis loops.

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10.1038/srep08595

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title = "Giant strain with ultra-low hysteresis and high temperature stability in grain oriented lead-free K 0.5 Bi 0.5 TiO3-BaTiO3-Na0.5 Bi0.5 TiO3 piezoelectric materials",

abstract = "We synthesized grain-oriented lead-free piezoelectric materials in (K 0.5 Bi 0.5 TiO3-BaTiO3-Na0.5 Bi0.5 TiO3 (KBT-BT-NBT) system with high degree of texturing along the [001]c (c-cubic) crystallographic orientation. We demonstrate giant field induced strain (∼0.48%) with an ultra-low hysteresis along with enhanced piezoelectric response (d 33 ∼ 190pC/N) and high temperature stability (∼160°C). Transmission electron microscopy (TEM) and piezoresponse force microscopy (PFM) results demonstrate smaller size highly ordered domain structure in grain-oriented specimen relative to the conventional polycrystalline ceramics. The grain oriented specimens exhibited a high degree of non-180° domain switching, in comparison to the randomly axed ones. These results indicate the effective solution to the lead-free piezoelectric materials.",

author = "Deepam Maurya and Yuan Zhou and Yaojin Wang and Yongke Yan and Jiefang Li and Dwight Viehland and Shashank Priya",

note = "Funding Information: The authors gratefully acknowledge financial support from the Office of Basic Energy Science, Department of Energy through grant number DE-FG02-07ER46480. Thanks to Keyur B. Joshi for his help in calculating dissipated energy from the P-E hysteresis loops.",

year = "2015",

doi = "10.1038/srep08595",

language = "English (US)",

volume = "5",

journal = "Scientific reports",

issn = "2045-2322",

publisher = "Nature Publishing Group",

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T1 - Giant strain with ultra-low hysteresis and high temperature stability in grain oriented lead-free K 0.5 Bi 0.5 TiO3-BaTiO3-Na0.5 Bi0.5 TiO3 piezoelectric materials

AU - Maurya, Deepam

AU - Zhou, Yuan

AU - Wang, Yaojin

AU - Yan, Yongke

AU - Li, Jiefang

AU - Viehland, Dwight

AU - Priya, Shashank

N1 - Funding Information: The authors gratefully acknowledge financial support from the Office of Basic Energy Science, Department of Energy through grant number DE-FG02-07ER46480. Thanks to Keyur B. Joshi for his help in calculating dissipated energy from the P-E hysteresis loops.

PY - 2015

Y1 - 2015

N2 - We synthesized grain-oriented lead-free piezoelectric materials in (K 0.5 Bi 0.5 TiO3-BaTiO3-Na0.5 Bi0.5 TiO3 (KBT-BT-NBT) system with high degree of texturing along the [001]c (c-cubic) crystallographic orientation. We demonstrate giant field induced strain (∼0.48%) with an ultra-low hysteresis along with enhanced piezoelectric response (d 33 ∼ 190pC/N) and high temperature stability (∼160°C). Transmission electron microscopy (TEM) and piezoresponse force microscopy (PFM) results demonstrate smaller size highly ordered domain structure in grain-oriented specimen relative to the conventional polycrystalline ceramics. The grain oriented specimens exhibited a high degree of non-180° domain switching, in comparison to the randomly axed ones. These results indicate the effective solution to the lead-free piezoelectric materials.

AB - We synthesized grain-oriented lead-free piezoelectric materials in (K 0.5 Bi 0.5 TiO3-BaTiO3-Na0.5 Bi0.5 TiO3 (KBT-BT-NBT) system with high degree of texturing along the [001]c (c-cubic) crystallographic orientation. We demonstrate giant field induced strain (∼0.48%) with an ultra-low hysteresis along with enhanced piezoelectric response (d 33 ∼ 190pC/N) and high temperature stability (∼160°C). Transmission electron microscopy (TEM) and piezoresponse force microscopy (PFM) results demonstrate smaller size highly ordered domain structure in grain-oriented specimen relative to the conventional polycrystalline ceramics. The grain oriented specimens exhibited a high degree of non-180° domain switching, in comparison to the randomly axed ones. These results indicate the effective solution to the lead-free piezoelectric materials.

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