Abstract
It is a distinct possibility that spin fluctuations are the pairing interactions in numerous unconventional superconductors. In the high-transition-temperature (high-Tc) cuprates, superconductivity emerges upon doping antiferromagnetic Mott insulators, and spin fluctuations might furthermore drive unusual pseudogap phenomena. Here we use magnetic neutron scattering to study the highly underdoped cuprate HgBa2CuO4+δ (hole concentration p ≈ 0.064). In contrast to prior results for other underdoped cuprates, we find no evidence of incommensurate magnetic order associated with spin-density-wave or stripe correlations. Instead, the antiferromagnetic response in both the superconducting and pseudogap states is gapped below ΔAF ≈ 6 meV, commensurate over a wide energy range, and disperses above about 55 meV. Given the pristine nature of HgBa2CuO4+δ, which exhibits high structural symmetry and minimal point disorder effects, this behavior likely signifies the unmasked response of the underlying CuO2 planes near the Mott-insulating state. These results serve as a benchmark for a refined theoretical understanding of the cuprates.
| Original language | English (US) |
|---|---|
| Article number | 93 |
| Journal | npj Quantum Materials |
| Volume | 10 |
| Issue number | 1 |
| DOIs | |
| State | Published - Dec 2025 |
Bibliographical note
Publisher Copyright:© The Author(s) 2025.