Comparative study on characteristics of the bio-oil from microwave-assisted pyrolysis of lignocellulose and triacylglycerol

Leilei Dai; Yunpu Wang; Yuhuan Liu; Roger Ruan; Zhenting Yu; Lin Jiang

doi:10.1016/j.scitotenv.2018.12.241

Comparative study on characteristics of the bio-oil from microwave-assisted pyrolysis of lignocellulose and triacylglycerol

Leilei Dai, Yunpu Wang, Yuhuan Liu, Roger Ruan, Zhenting Yu, Lin Jiang

Bioproducts and Biosystems Engineering

Research output: Contribution to journal › Article › peer-review

33 Scopus citations

Abstract

Microwave-assisted pyrolysis of Camellia oleifera shell (COS) and stillingia oil (SO) was performed in the temperature range of 400–600 °C. The effects of feedstock and pyrolysis temperatures on product yield and bio-oil composition were discussed in detail. The bio-oil yield from COS pyrolysis varied from 37.30 wt% to 40.27 wt%, which was 11.32 wt% to 21.62 wt% lower than that from SO pyrolysis. Gas chromatography–mass spectrometry analysis indicated that SO bio-oil was rich in hydrocarbons, whereas COS pyrolysis produced mainly oxygen-containing compounds predominantly comprising phenols and acids. Fourier transform infrared and ¹H-nuclear magnetic resonance spectra showed significant differences in the chemical structure of bio-oils from COS and SO pyrolysis. Elemental-composition and physical-property analyses further revealed that SO bio-oils were similar to gasoline and heavy fuel oil.

Original language	English (US)
Pages (from-to)	95-100
Number of pages	6
Journal	Science of the Total Environment
Volume	659
DOIs	https://doi.org/10.1016/j.scitotenv.2018.12.241
State	Published - Apr 1 2019

Bibliographical note

Funding Information:
This project is financially supported by the National Natural Science Foundation of China (No. 21766019, 21878137), Natural Science Foundation of Jiangxi Province (20181BAB206030), Research Project of State Key Laboratory of Food Science and Technology (SKLF-ZZB-201722), Key Research and Development Program of Jiangxi Province (20171BBF60023), Science and Technology Research Project of Jiangxi Provincial Education Department (No. GJJ150213), Guangdong Provincial Key Laboratory of New and Renewable Energy Research and Development (No. Y707sb1001), Graduate Student Innovation Project (YC2017-S067, CX2017159), Innovation and Entrepreneurship Development Fund of “One Thousand Program” Talent (No. 1001-02102082).

Funding Information:
This project is financially supported by the National Natural Science Foundation of China (No. 21766019, 21878137 ), Natural Science Foundation of Jiangxi Province ( 20181BAB206030 ), Research Project of State Key Laboratory of Food Science and Technology ( SKLF-ZZB-201722 ), Key Research and Development Program of Jiangxi Province ( 20171BBF60023 ), Science and Technology Research Project of Jiangxi Provincial Education Department (No. GJJ150213 ), Guangdong Provincial Key Laboratory of New and Renewable Energy Research and Development (No. Y707sb1001 ), Graduate Student Innovation Project ( YC2017-S067 , CX2017159 ), Innovation and Entrepreneurship Development Fund of “One Thousand Program” Talent (No. 1001-02102082 ).

Publisher Copyright:
© 2018

Keywords

Bio-oil
Lignocellulose
Microwave-assisted pyrolysis
Triacylglycerol

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10.1016/j.scitotenv.2018.12.241

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title = "Comparative study on characteristics of the bio-oil from microwave-assisted pyrolysis of lignocellulose and triacylglycerol",

abstract = "Microwave-assisted pyrolysis of Camellia oleifera shell (COS) and stillingia oil (SO) was performed in the temperature range of 400–600 °C. The effects of feedstock and pyrolysis temperatures on product yield and bio-oil composition were discussed in detail. The bio-oil yield from COS pyrolysis varied from 37.30 wt% to 40.27 wt%, which was 11.32 wt% to 21.62 wt% lower than that from SO pyrolysis. Gas chromatography–mass spectrometry analysis indicated that SO bio-oil was rich in hydrocarbons, whereas COS pyrolysis produced mainly oxygen-containing compounds predominantly comprising phenols and acids. Fourier transform infrared and 1H-nuclear magnetic resonance spectra showed significant differences in the chemical structure of bio-oils from COS and SO pyrolysis. Elemental-composition and physical-property analyses further revealed that SO bio-oils were similar to gasoline and heavy fuel oil.",

keywords = "Bio-oil, Lignocellulose, Microwave-assisted pyrolysis, Triacylglycerol",

author = "Leilei Dai and Yunpu Wang and Yuhuan Liu and Roger Ruan and Zhenting Yu and Lin Jiang",

note = "Funding Information: This project is financially supported by the National Natural Science Foundation of China (No. 21766019, 21878137), Natural Science Foundation of Jiangxi Province (20181BAB206030), Research Project of State Key Laboratory of Food Science and Technology (SKLF-ZZB-201722), Key Research and Development Program of Jiangxi Province (20171BBF60023), Science and Technology Research Project of Jiangxi Provincial Education Department (No. GJJ150213), Guangdong Provincial Key Laboratory of New and Renewable Energy Research and Development (No. Y707sb1001), Graduate Student Innovation Project (YC2017-S067, CX2017159), Innovation and Entrepreneurship Development Fund of “One Thousand Program” Talent (No. 1001-02102082). Funding Information: This project is financially supported by the National Natural Science Foundation of China (No. 21766019, 21878137 ), Natural Science Foundation of Jiangxi Province ( 20181BAB206030 ), Research Project of State Key Laboratory of Food Science and Technology ( SKLF-ZZB-201722 ), Key Research and Development Program of Jiangxi Province ( 20171BBF60023 ), Science and Technology Research Project of Jiangxi Provincial Education Department (No. GJJ150213 ), Guangdong Provincial Key Laboratory of New and Renewable Energy Research and Development (No. Y707sb1001 ), Graduate Student Innovation Project ( YC2017-S067 , CX2017159 ), Innovation and Entrepreneurship Development Fund of “One Thousand Program” Talent (No. 1001-02102082 ). Publisher Copyright: {\textcopyright} 2018",

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AU - Dai, Leilei

AU - Wang, Yunpu

AU - Liu, Yuhuan

AU - Ruan, Roger

AU - Yu, Zhenting

AU - Jiang, Lin

N1 - Funding Information: This project is financially supported by the National Natural Science Foundation of China (No. 21766019, 21878137), Natural Science Foundation of Jiangxi Province (20181BAB206030), Research Project of State Key Laboratory of Food Science and Technology (SKLF-ZZB-201722), Key Research and Development Program of Jiangxi Province (20171BBF60023), Science and Technology Research Project of Jiangxi Provincial Education Department (No. GJJ150213), Guangdong Provincial Key Laboratory of New and Renewable Energy Research and Development (No. Y707sb1001), Graduate Student Innovation Project (YC2017-S067, CX2017159), Innovation and Entrepreneurship Development Fund of “One Thousand Program” Talent (No. 1001-02102082). Funding Information: This project is financially supported by the National Natural Science Foundation of China (No. 21766019, 21878137 ), Natural Science Foundation of Jiangxi Province ( 20181BAB206030 ), Research Project of State Key Laboratory of Food Science and Technology ( SKLF-ZZB-201722 ), Key Research and Development Program of Jiangxi Province ( 20171BBF60023 ), Science and Technology Research Project of Jiangxi Provincial Education Department (No. GJJ150213 ), Guangdong Provincial Key Laboratory of New and Renewable Energy Research and Development (No. Y707sb1001 ), Graduate Student Innovation Project ( YC2017-S067 , CX2017159 ), Innovation and Entrepreneurship Development Fund of “One Thousand Program” Talent (No. 1001-02102082 ). Publisher Copyright: © 2018

PY - 2019/4/1

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N2 - Microwave-assisted pyrolysis of Camellia oleifera shell (COS) and stillingia oil (SO) was performed in the temperature range of 400–600 °C. The effects of feedstock and pyrolysis temperatures on product yield and bio-oil composition were discussed in detail. The bio-oil yield from COS pyrolysis varied from 37.30 wt% to 40.27 wt%, which was 11.32 wt% to 21.62 wt% lower than that from SO pyrolysis. Gas chromatography–mass spectrometry analysis indicated that SO bio-oil was rich in hydrocarbons, whereas COS pyrolysis produced mainly oxygen-containing compounds predominantly comprising phenols and acids. Fourier transform infrared and 1H-nuclear magnetic resonance spectra showed significant differences in the chemical structure of bio-oils from COS and SO pyrolysis. Elemental-composition and physical-property analyses further revealed that SO bio-oils were similar to gasoline and heavy fuel oil.

AB - Microwave-assisted pyrolysis of Camellia oleifera shell (COS) and stillingia oil (SO) was performed in the temperature range of 400–600 °C. The effects of feedstock and pyrolysis temperatures on product yield and bio-oil composition were discussed in detail. The bio-oil yield from COS pyrolysis varied from 37.30 wt% to 40.27 wt%, which was 11.32 wt% to 21.62 wt% lower than that from SO pyrolysis. Gas chromatography–mass spectrometry analysis indicated that SO bio-oil was rich in hydrocarbons, whereas COS pyrolysis produced mainly oxygen-containing compounds predominantly comprising phenols and acids. Fourier transform infrared and 1H-nuclear magnetic resonance spectra showed significant differences in the chemical structure of bio-oils from COS and SO pyrolysis. Elemental-composition and physical-property analyses further revealed that SO bio-oils were similar to gasoline and heavy fuel oil.

KW - Bio-oil

KW - Lignocellulose

KW - Microwave-assisted pyrolysis

KW - Triacylglycerol

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AN - SCOPUS:85059199261

SN - 0048-9697

VL - 659

SP - 95

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JO - Science of the Total Environment

JF - Science of the Total Environment

ER -

Comparative study on characteristics of the bio-oil from microwave-assisted pyrolysis of lignocellulose and triacylglycerol

Abstract

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