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2017

505623 microporous inorganic and composite membranes for energy efficient separations

Tsapatsis, M. & Lin, J., Jan 1 2017, Meet the Faculty Candidate Poster Session 2017 � Sponsored by the Education Division - Topical Conference at the 2017 AIChE Annual Meeting. AIChE, Vol. 2017-October. p. 263-264 2 p.

Research output: Chapter in Book/Report/Conference proceedingConference contribution

Composite membranes
4 Citations

A review of biorefinery separations for bioproduct production via thermocatalytic processing

Nguyen, H., Dejaco, R. F., Mittal, N., Siepmann, J. I., Tsapatsis, M., Snyder, M. A., Fan, W., Saha, B. & Vlachos, D. G., Jun 7 2017, In : Annual Review of Chemical and Biomolecular Engineering. 8, p. 115-137 23 p.

Research output: Contribution to journalReview article

Processing
Biomass
Carbon
Zeolites
Adsorption
3 Citations
economic analysis
Zeolites
Bioethanol
Molecular modeling
Economic analysis
9 Citations

Biomass-Derived Butadiene by Dehydra-Decyclization of Tetrahydrofuran

Abdelrahman, O. A., Park, D. S., Vinter, K. P., Spanjers, C. S., Ren, L., Cho, H. J., Vlachos, D. G., Fan, W., Tsapatsis, M. & Dauenhauer, P. J., May 1 2017, In : ACS Sustainable Chemistry and Engineering. 5, 5, p. 3732-3736 5 p.

Research output: Contribution to journalArticle

Butadiene
Phosphorus
Biomass
phosphorus
Furfural
3 Citations

Epitaxial growth: Rapid synthesis of highly permeable and selective zeolite-T membranes

Luo, Y., Lv, Y., Kumar, P., Chu, J., Yang, J., Tsapatsis, M., Mkhoyan, K. A., He, G., Lu, J. & Zhang, Y., Jan 1 2017, In : Journal of Materials Chemistry A. 5, 34, p. 17828-17832 5 p.

Research output: Contribution to journalArticle

Zeolites
Epitaxial growth
Seed
Membranes
2-Propanol
35 Citations

Hydrogen Sulfide Capture: From Absorption in Polar Liquids to Oxide, Zeolite, and Metal-Organic Framework Adsorbents and Membranes

Shah, M. S., Tsapatsis, M. & Siepmann, J. I., Jul 26 2017, In : Chemical Reviews. 117, 14, p. 9755-9803 49 p.

Research output: Contribution to journalReview article

Zeolites
Hydrogen Sulfide
Adsorbents
Oxides
Metals
13 Citations

Nanoscale Control of Homoepitaxial Growth on a Two-Dimensional Zeolite

Shete, M., Kumar, M., Kim, D., Rangnekar, N., Xu, D., Topuz, B., Agrawal, K. V., Karapetrova, E., Stottrup, B., Al-Thabaiti, S., Basahel, S., Narasimharao, K., Rimer, J. D. & Tsapatsis, M., Jan 1 2017, In : Angewandte Chemie - International Edition. 56, 2, p. 535-539 5 p.

Research output: Contribution to journalArticle

Zeolites
Crystal growth
Crystallization
Nanosheets
Crystallites
12 Citations

Renewable Isoprene by Sequential Hydrogenation of Itaconic Acid and Dehydra-Decyclization of 3-Methyl-Tetrahydrofuran

Abdelrahman, O. A., Park, D. S., Vinter, K. P., Spanjers, C. S., Ren, L., Cho, H. J., Zhang, K., Fan, W., Tsapatsis, M. & Dauenhauer, P. J., Feb 3 2017, In : ACS Catalysis. 7, 2, p. 1428-1431 4 p.

Research output: Contribution to journalArticle

Isoprene
Hydrogenation
Acids
Alkadienes
Zeolites
22 Citations

Renewable p-Xylene from 2,5-Dimethylfuran and Ethylene Using Phosphorus-Containing Zeolite Catalysts

Cho, H. J., Ren, L., Vattipalli, V., Yeh, Y. H., Gould, N., Xu, B., Gorte, R. J., Lobo, R., Dauenhauer, P. J., Tsapatsis, M. & Fan, W., Feb 6 2017, In : ChemCatChem. 9, 3, p. 398-402 5 p.

Research output: Contribution to journalArticle

Zeolites
xylene
Xylene
Phosphorus
phosphorus
5 Citations

Simple quantification of zeolite acid site density by reactive gas chromatography

Abdelrahman, O. A., Vinter, K. P., Ren, L., Xu, D., Gorte, R. J., Tsapatsis, M. & Dauenhauer, P. J., Jan 1 2017, In : Catalysis Science and Technology. 7, 17, p. 3831-3841 11 p.

Research output: Contribution to journalArticle

Zeolites
Gas chromatography
Acids
Gases
Temperature programmed desorption
4 Citations

Studying two-dimensional zeolites with the tools of surface science: MFI nanosheets on Au(111)

Kestell, J. D., Zhong, J. Q., Shete, M., Waluyo, I., Sadowski, J. T., Stacchiola, D. J., Tsapatsis, M. & Boscoboinik, J. A., Feb 1 2017, In : Catalysis Today. 280, p. 283-288 6 p.

Research output: Contribution to journalArticle

Zeolites
Nanosheets
Absorption spectroscopy
Infrared radiation
Catalysts
1 Citations

Sub-Micrometer Zeolite Films on Gold-Coated Silicon Wafers with Single-Crystal-Like Dielectric Constant and Elastic Modulus

Tiriolo, R., Rangnekar, N., Zhang, H., Shete, M., Bai, P., Nelson, J., Karapetrova, E., Macosko, C. W., Siepmann, J. I., Lamanna, E., Lavano, A. & Tsapatsis, M., Jul 5 2017, In : Advanced Functional Materials. 27, 25, 1700864.

Research output: Contribution to journalArticle

Zeolites
Silicon wafers
Gold
micrometers
modulus of elasticity
4 Citations

Transferable potentials for phase equilibria. Improved united-atom description of ethane and ethylene

Shah, M. S., Siepmann, J. I. & Tsapatsis, M., Nov 1 2017, In : AIChE Journal. 63, 11, p. 5098-5110 13 p.

Research output: Contribution to journalArticle

Ethane
Phase equilibria
Ethylene
Atoms
Vapor Pressure
57 Citations

Ultra-selective high-flux membranes from directly synthesized zeolite nanosheets

Jeon, M. Y., Kim, D., Kumar, P., Lee, P. S., Rangnekar, N., Bai, P., Shete, M., Elyassi, B., Lee, H. S., Narasimharao, K., Basahel, S. N., Al-Thabaiti, S., Xu, W., Cho, H. J., Fetisov, E. O., Thyagarajan, R., Dejaco, R. F., Fan, W., Mkhoyan, K. A., Siepmann, J. I. & 1 othersTsapatsis, M., Mar 30 2017, In : Nature. 543, 7647, p. 690-694 5 p.

Research output: Contribution to journalArticle

Zeolites
Membranes
Nanoparticles
Chemical Industry
Silicates
2016
12 Citations

Adsorptive Separation of 1-Butanol from Aqueous Solutions Using MFI-and FER-Type Zeolite Frameworks: A Monte Carlo Study

Dejaco, R. F., Bai, P., Tsapatsis, M. & Siepmann, J. I., Mar 1 2016, In : Langmuir. 32, 8, p. 2093-2101 9 p.

Research output: Contribution to journalArticle

Zeolites
1-Butanol
Butenes
sorbates
ethyl alcohol
7 Citations
Zeolites
Distillation
distillation
Butane
butanes
9 Citations

Combining Pre- and Post-Nucleation Trajectories for the Synthesis of High FAU-Content Faujasite Nanocrystals from Organic-Free Sols

Khaleel, M., Xu, W., Lesch, D. A. & Tsapatsis, M., Jun 28 2016, In : Chemistry of Materials. 28, 12, p. 4204-4213 10 p.

Research output: Contribution to journalArticle

Polymethyl Methacrylate
Sols
Nanocrystals
Nucleation
Trajectories

Cover Picture: Open-Pore Two-Dimensional MFI Zeolite Nanosheets for the Fabrication of Hydrocarbon-Isomer-Selective Membranes on Porous Polymer Supports (Angew. Chem. Int. Ed. 25/2016)

Zhang, H., Xiao, Q., Guo, X., Li, N., Kumar, P., Rangnekar, N., Jeon, M. Y., Al-Thabaiti, S., Narasimharao, K., Basahel, S. N., Topuz, B., Onorato, F. J., Macosko, C. W., Mkhoyan, K. A. & Tsapatsis, M., Jan 1 2016, In : Angewandte Chemie - International Edition. 55, 25, 1 p.

Research output: Contribution to journalComment/debate

Zeolites
Nanosheets
Hydrocarbons
Isomers
Polymers
19 Citations

Ethanol/water mixture pervaporation performance of b-oriented silicalite-1 membranes made by gel-free secondary growth

Elyassi, B., Jeon, M. Y., Tsapatsis, M., Narasimharao, K., Basahel, S. N. & Al-Thabaiti, S., Feb 1 2016, In : AICHE Journal. 62, 2, p. 556-563 8 p.

Research output: Contribution to journalArticle

Pervaporation
Ethanol
Gels
Silicon Dioxide
Membranes
11 Citations

Factors Governing the Formation of Hierarchically and Sequentially Intergrown MFI Zeolites by Using Simple Diquaternary Ammonium Structure-Directing Agents

Keoh, S. H., Chaikittisilp, W., Muraoka, K., Mukti, R. R., Shimojima, A., Kumar, P., Tsapatsis, M. & Okubo, T., Dec 27 2016, In : Chemistry of Materials. 28, 24, p. 8997-9007 11 p.

Research output: Contribution to journalArticle

Diquat
Zeolites
Ammonium Compounds
Crystals
Electron microscopes
3 Citations

Hierarchical materials: Background and perspectives

Mishnaevsky, L. & Tsapatsis, M., Sep 1 2016, In : MRS Bulletin. 41, 9, p. 661-664 4 p.

Research output: Contribution to journalArticle

inspiration
nanotechnology
manufacturing
requirements
Nanotechnology
8 Citations

Identifying Optimal Zeolitic Sorbents for Sweetening of Highly Sour Natural Gas

Shah, M. S., Tsapatsis, M. & Siepmann, J. I., May 10 2016, In : Angewandte Chemie - International Edition. 55, 20, p. 5938-5942 5 p.

Research output: Contribution to journalArticle

Hydrocarbons
Sorbents
Natural gas
Sour gas
Zeolites
14 Citations

Interplay between hydrophilicity and surface barriers on water transport in zeolite membranes

Fasano, M., Humplik, T., Bevilacqua, A., Tsapatsis, M., Chiavazzo, E., Wang, E. N. & Asinari, P., Oct 3 2016, In : Nature communications. 7, 12762.

Research output: Contribution to journalArticle

Zeolites
Hydrophilicity
Hydrophobic and Hydrophilic Interactions
Permeability
Nanopores
6 Citations

Modeling, optimization, and cost analysis of an IGCC plant with a membrane reactor for carbon capture

Lima, F. V., Daoutidis, P. & Tsapatsis, M., May 1 2016, In : AIChE Journal. 62, 5, p. 1568-1580 13 p.

Research output: Contribution to journalArticle

Carbon capture
Gasification
Carbon
Membranes
Costs and Cost Analysis
12 Citations

Nucleation of open framework materials: Navigating the voids

Rimer, J. D. & Tsapatsis, M., May 1 2016, In : MRS Bulletin. 41, 5, p. 393-398 6 p.

Research output: Contribution to journalReview article

voids
Nucleation
nucleation
crystals
Crystal engineering
24 Citations

Open-Pore Two-Dimensional MFI Zeolite Nanosheets for the Fabrication of Hydrocarbon-Isomer-Selective Membranes on Porous Polymer Supports

Zhang, H., Xiao, Q., Guo, X., Li, N., Kumar, P., Rangnekar, N., Jeon, M. Y., Al-Thabaiti, S., Narasimharao, K., Basahel, S. N., Topuz, B., Onorato, F. J., Macosko, C. W., Mkhoyan, K. A. & Tsapatsis, M., Jan 1 2016, In : Angewandte Chemie - International Edition. 55, 25, p. 7184-7187 4 p.

Research output: Contribution to journalArticle

Zeolites
Nanosheets
Butane
Hydrocarbons
Isomers
11 Citations

Oxidation and Reduction under Cover: Chemistry at the Confined Space between Ultrathin Nanoporous Silicates and Ru(0001)

Zhong, J. Q., Kestell, J., Waluyo, I., Wilkins, S., Mazzoli, C., Barbour, A., Kaznatcheev, K., Shete, M., Tsapatsis, M. & Boscoboinik, J. A., May 5 2016, In : Journal of Physical Chemistry C. 120, 15, p. 8240-8245 6 p.

Research output: Contribution to journalArticle

Silicates
Silicon Dioxide
silicates
Silica
chemistry
8 Citations

Pillared Sn-MWW Prepared by a Solid-State-Exchange Method and its Use as a Lewis Acid Catalyst

Ren, L., Guo, Q., Orazov, M., Xu, D., Politi, D., Kumar, P., Alhassan, S. M., Mkhoyan, K. A., Sidiras, D., Davis, M. E. & Tsapatsis, M., Apr 6 2016, In : ChemCatChem. 8, 7, p. 1274-1278 5 p.

Research output: Contribution to journalArticle

Lewis Acids
solid state
catalysts
acids
Catalysts
25 Citations

Thermal Stabilization of Metal-Organic Framework-Derived Single-Site Catalytic Clusters through Nanocasting

Malonzo, C. D., Shaker, S. M., Ren, L., Prinslow, S. D., Platero-Prats, A. E., Gallington, L. C., Borycz, J., Thompson, A. B., Wang, T. C., Farha, O. K., Hupp, J. T., Lu, C. C., Chapman, K. W., Myers, J. C., Penn, R. L., Gagliardi, L., Tsapatsis, M. & Stein, A., Mar 2 2016, In : Journal of the American Chemical Society. 138, 8, p. 2739-2748 10 p.

Research output: Contribution to journalArticle

Catalytic Domain
Stabilization
Hot Temperature
Metals
Silicon Dioxide
7 Citations

Tunable oleo-furan surfactants by acylation of renewable furans

Park, D. S., Joseph, K. E., Koehle, M., Krumm, C., Ren, L., Damen, J. N., Shete, M. H., Lee, H. S., Zuo, X., Lee, B., Fan, W., Vlachos, D. G., Lobo, R. F., Tsapatsis, M. & Dauenhauer, P. J., Nov 23 2016, In : ACS Central Science. 2, 11, p. 820-824 5 p.

Research output: Contribution to journalArticle

Furans
Acylation
Surface-Active Agents
Surface active agents
Water
12 Citations

Understanding Diffusion in Hierarchical Zeolites with House-of-Cards Nanosheets

Bai, P., Haldoupis, E., Dauenhauer, P. J., Tsapatsis, M. & Siepmann, J. I., Aug 23 2016, In : ACS Nano. 10, 8, p. 7612-7618 7 p.

Research output: Contribution to journalArticle

Zeolites
Nanosheets
zeolites
sorbates
free energy
2015
27 Citations

2D zeolite coatings: Langmuir-Schaefer deposition of 3 nm thick MFI zeolite nanosheets

Rangnekar, N., Shete, M., Agrawal, K. V., Topuz, B., Kumar, P., Guo, Q., Ismail, I., Alyoubi, A., Basahel, S., Narasimharao, K., Macosko, C. W., Mkhoyan, K. A., Al-Thabaiti, S., Stottrup, B. & Tsapatsis, M., May 1 2015, In : Angewandte Chemie - International Edition. 54, 22, p. 6571-6575 5 p.

Research output: Contribution to journalArticle

Zeolites
Nanosheets
Coatings
Calcination
Suspensions

431787 a highly permeable and selective aminofunctionalized MOF CAU-1 membrane for separation of molecular mixture

Yang, J., Yin, H., Wang, J., Lu, J., Zhang, Y., Lin, J. Y. S. & Tsapatsis, M., Jan 1 2015, Separations Division 2015 - Core Programming Area at the 2015 AIChE Annual Meeting. AIChE, Vol. 2. p. 753-755 3 p.

Research output: Chapter in Book/Report/Conference proceedingConference contribution

Membranes
Adsorption
Pore size
Gases
Metals
4 Citations

Activation of giant silicalite-1 monocrystals combining rapid thermal processing and ozone calcination

Navarro, M., Mateo, E., Diosdado, B., Tsapatsis, M. & Coronas, J., Jan 1 2015, In : RSC Advances. 5, 23, p. 18035-18040 6 p.

Research output: Contribution to journalArticle

Rapid thermal processing
Ozone
Calcination
Thermogravimetric analysis
Chemical activation
7 Citations

Carbon Nanotube Selective Membranes with Subnanometer, Vertically Aligned Pores, and Enhanced Gas Transport Properties

Labropoulos, A., Veziri, C., Kapsi, M., Pilatos, G., Likodimos, V., Tsapatsis, M., Kanellopoulos, N. K., Romanos, G. E. & Karanikolos, G. N., Dec 22 2015, In : Chemistry of Materials. 27, 24, p. 8198-8210 13 p.

Research output: Contribution to journalArticle

Carbon Nanotubes
Transport properties
Nanotubes
Carbon nanotubes
Gases
17 Citations

Development of the Transferable Potentials for Phase Equilibria Model for Hydrogen Sulfide

Shah, M. S., Tsapatsis, M. & Siepmann, J. I., Jun 11 2015, In : Journal of Physical Chemistry B. 119, 23, p. 7041-7052 12 p.

Research output: Contribution to journalArticle

Hydrogen Sulfide
hydrogen sulfide
Hydrogen sulfide
Phase equilibria
Atoms
41 Citations

Discovery of optimal zeolites for challenging separations and chemical transformations using predictive materials modeling

Bai, P., Jeon, M. Y., Ren, L., Knight, C., Deem, M. W., Tsapatsis, M. & Siepmann, J. I., Jan 21 2015, In : Nature communications. 6, 5912.

Research output: Contribution to journalArticle

Zeolites
crude oil
zeolites
broths
fermentation
3 Citations

Economic assessment of Temperature Swing Adsorption systems as Claus Tail Gas Clean Up Units

Al Wahedi, Y., Torres, A. I., Al Hashimi, S., Dowling, N. I., Daoutidis, P. & Tsapatsis, M., Apr 4 2015, In : Chemical Engineering Science. 126, p. 186-195 10 p.

Research output: Contribution to journalArticle

Gases
Sulfur
Adsorption
Recovery
Economics
9 Citations

Monte Carlo simulations probing the adsorptive separation of hydrogen sulfide/methane mixtures using all-silica zeolites

Shah, M. S., Tsapatsis, M. & Siepmann, J. I., Nov 10 2015, In : Langmuir. 31, 44, p. 12268-12278 11 p.

Research output: Contribution to journalArticle

Zeolites
Hydrogen Sulfide
hydrogen sulfide
Methane
Hydrogen sulfide
4 Citations

Nucleation, Growth, and Robust Synthesis of SPP Zeolite: Effect of Ethanol, Sodium, and Potassium

Swindlehurst, G. R., Kumar, P., Xu, D., Alhassan, S. M., Mkhoyan, K. A. & Tsapatsis, M., May 28 2015, In : Topics in Catalysis. 58, 7-9, p. 545-558 14 p.

Research output: Contribution to journalArticle

Zeolites
Nanosheets
Polymethyl Methacrylate
Sols
Potassium
53 Citations

Oriented MFI membranes by gel-less secondary growth of sub-100 nm MFI-nanosheet seed layers

Agrawal, K. V., Topuz, B., Pham, T. C. T., Nguyen, T. H., Sauer, N., Rangnekar, N., Zhang, H., Narasimharao, K., Basahel, S. N., Francis, L. F., Macosko, C. W., Al-Thabaiti, S., Tsapatsis, M. & Yoon, K. B., Jun 1 2015, In : Advanced Materials. 27, 21, p. 3243-3249 7 p.

Research output: Contribution to journalArticle

Zeolites
Nanosheets
Molecular sieves
Butane
Xylene
15 Citations

Quantification of thickness and wrinkling of exfoliated two-dimensional zeolite nanosheets

Kumar, P., Agrawal, K. V., Tsapatsis, M. & Mkhoyan, K. A., May 11 2015, In : Nature communications. 6, 7128.

Research output: Contribution to journalArticle

wrinkling
Zeolites
Nanosheets
Silicates
Molecular sieves
57 Citations

Self-Pillared, Single-Unit-Cell Sn-MFI Zeolite Nanosheets and Their Use for Glucose and Lactose Isomerization

Ren, L., Guo, Q., Kumar, P., Orazov, M., Xu, D., Alhassan, S. M., Mkhoyan, K. A., Davis, M. E. & Tsapatsis, M., Sep 1 2015, In : Angewandte Chemie - International Edition. 54, 37, p. 10848-10851 4 p.

Research output: Contribution to journalArticle

Lactulose
Zeolites
Fructose
Nanosheets
Lactose
1 Citations

Techno-economic analysis of ethanol-selective membranes for corn ethanol-water separation

Kelloway, A., Tsapatsis, M. & Daoutidis, P., Jan 1 2015, In : Computer Aided Chemical Engineering. 37, p. 365-370 6 p.

Research output: Contribution to journalArticle

Economic analysis
Ethanol
Membranes
Water
Distillation
148 Citations

Zeolite membranes - a review and comparison with MOFs

Rangnekar, N., Mittal, N., Elyassi, B., Caro, J. & Tsapatsis, M., Oct 21 2015, In : Chemical Society Reviews. 44, 20, p. 7128-7154 27 p.

Research output: Contribution to journalReview article

Zeolites
Membranes
Metals
Industrial applications
Seed
2014
44 Citations

2-dimensional zeolites

Tsapatsis, M., Jan 1 2014, In : AICHE Journal. 60, 7, p. 2374-2381 8 p.

Research output: Contribution to journalArticle

Zeolites
Catalysis
Membranes
14 Citations
Zeolites
Alkylation
zeolites
selectivity
Titration
26 Citations

A high-performance adsorbent for hydrogen sulfide removal

Elyassi, B., Wahedi, Y. A., Rajabbeigi, N., Kumar, P., Jeong, J. S., Zhang, X., Kumar, P., Balasubramanian, V. V., Katsiotis, M. S., Andre Mkhoyan, K., Boukos, N., Hashimi, S. A. & Tsapatsis, M., May 15 2014, In : Microporous and Mesoporous Materials. 190, p. 152-155 4 p.

Research output: Contribution to journalArticle

hydrogen sulfide
adsorbents
Adsorbents
Zinc Oxide
Adsorption
46 Citations

Challenges of and Insights into Acid-Catalyzed Transformations of Sugars

Caratzoulas, S., Davis, M. E., Gorte, R. J., Gounder, R., Lobo, R. F., Nikolakis, V., Sandler, S. I., Snyder, M. A., Tsapatsis, M. & Vlachos, D. G., Oct 9 2014, In : Journal of Physical Chemistry C. 118, 40, p. 22815-22833 19 p.

Research output: Contribution to journalArticle

Lewis Acids
sugars
Sugars
Hydroxyl Radical
acids
5 Citations
Zeolites
Isomers
Ethanol
ethyl alcohol
isomers